Aerosol impacts on post-monsoon meteorology in North India predicted by the Japan Meteorological Agency’s online-coupled meteorology–chemistry model NHM-Chem v2.0
DOI:
https://doi.org/10.51094/jxiv.3338キーワード:
Crop residue burning、 PM2.5、 Aerosol-to-meteorology feedback、 Model development、 Multi-model intercomparison抄録
The Japan Meteorological Agency’s online-coupled meteorology–chemistry model with aerosol-to-meteorology feedback, NHM-Chem v2.0, was developed and applied to post-monsoon air pollution episodes associated with Kharif crop residue burning (CRB) over North India in 2022. Model performance in simulating increases in surface concentrations of PM2.5 owing to aerosol–radiation feedback (referred to as “positive feedback”) were compared with those of WRF-Chem. Online NHM-Chem was 2.5 times faster than WRF-Chem, whereas WRF-Chem better reproduced spatiotemporal PM2.5 variations than NHM-Chem, probably because meteorological fields such as wind direction and planetary boundary layer (PBL) height predicted by WRF-Chem were generally more accurate than those from NHM-Chem. Both models successfully reproduced high PM2.5 episodes exceeding 300 µg m−3 caused by CRB plume transport under northwesterly winds, whereas the models failed to reproduce CRB plume transport during convective conditions. During the plume event (2–4 November), daytime solar radiation and PBL height decreased by 30%–40% and 50%–80%, respectively, increasing surface PM2.5 concentrations by up to 100% over the Delhi National Capital Region compared with clean-air scenarios. The contribution of CRB to surface PM2.5 varied from 40% to 80%, depending on the selection of models. Both model simulations indicated that CRB increased surface PM2.5 from anthropogenic and CRB sources equally by 15%–50% through positive feedback. Thus, discontinuing CRB would not only reduce CRB-related PM2.5 but also lower anthropogenic surface PM2.5 by 15%–50%.
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引用文献
Abdul-Razzak H, Ghan SJ (2000) A parameterization of aerosol activation 2. Multiple aerosol types. J Geophys Res Atmos 105(D5):6837-6844
Anand K A A, Ganguly D, Nandi I, Kajino M, Dey S (2025) Disentangling the separate and combined effects of aerosol-radiation and aerosol-photolysis interactions on air quality over India. J Geophys Res Atmos 130(24):e2025JD045316
Andersen ST, Carpenter LJ, Reed C, Lee JD, Chance R, Sherwen T, Vaughan AR, Stewart J, Edwards PM, Bloss WJ, Sommariva R, Crilley LR, Nott GJ, Neves L, Read K, Heard DE, Seakins PW, Whalley LK, Boustead GA, Fleming LT, Stone D, Fomba KW (2023) Extensive field evidence for the release of HONO from the photolysis of nitrate aerosols. Sci Adv 9:eadd6266
Bigg EK (1955) Ice‐crystal counts and the freezing of water drops. Q J R Meteorol Soc 81(349):478–479
Biswal A, Takigawa M, Mangaraj P, Bisht JSH, Patra PK, Matsumi Y, Nakayama T, Araki H, Yasutomi N, Singh V (2025) Emission time and amount of crop residue burning play critical role on PM2.5 variability during October–November in northwestern India during 2022–2024. Environ Sci Atmos 5(11):1211–1229
Bohren CF, Huffman DR (1983) Absorption and scattering of light by small particles. Wiley, New York
Briant R, Tuccella P, Deroubaix A, Khvorostyanov D, Menut L, Mailler S, Turquety S (2017) Aerosol-radiation interaction modelling using online coupling between the WRF 3.7.1 meteorological model and the CHIMERE 2016 chemistry-transport model, through the OASIS3-MCT coupler. Geosci Model Dev 10(2):927–944
Carter W (2000) Documentation of the SAPRC-99 chemical mechanism for VOC reactivity assessment, Final report to California Air Resources Board, Rep. 92-329, Univ. of Calif., Riverside, 8 May, 569 pp
Chen F, Dudhia J (2001) Coupling an advanced land surface–hydrology model with the Penn State–NCAR MM5 modeling system. Part I : Model implementation and sensitivity. Mon Wea Rev 129:569–585
Chin M, Ginoux P, Kinne S, Torres O, Holben BN, Duncan BN, Martin R V., Logan JA, Higurashi A, Nakajima T (2002) Tropospheric aerosol optical thickness from the GOCART model and comparisons with satellite and sun photometer measurements. J Atmos Sci 59:461–483.
Clarke AD, Owens SR, Zhou J (2006) An ultrafine sea-salt flux from breaking waves: Implications for cloud condensation nuclei in the remote marine atmosphere. J Geophys Res Atmos 111:D06202
Cusworth DH, Mickley LJ, Sulprizio MP, Liu T, Marlier ME, Ruth S (2018) Quantifying the influence of agricultural fires in northwest India on urban air pollution in Delhi, India. Environ Res Lett 13:044018
Deushi M, Shibata K (2011) Development of a Meteorological Research Institute chemistry-climate model version 2 for the study of tropospheric and stratospheric chemistry. Pap Meteorol Geophys 62:1–46
Fast JD, Gustafson WI, Easter RC, Zaveri RA, Barnard JC, Chapman EG, Grell GA, Peckham SE (2006) Evolution of ozone, particulates, and aerosol direct radiative forcing in the vicinity of Houston using a fully coupled meteorology-chemistry-aerosol model. J Geophys Res Atmos 111:D21305
Forkel R, Werhahn J, Hansen AB, McKeen S, Peckham S, Grell G, Suppan P (2012) Effect of aerosol-radiation feedback on regional air quality - A case study with WRF/Chem. Atmos Environ 53:202–211
Forster P, Storelvmo T, Armour K, Collins W, Dufresne JL, Frame D, Lunt DJ, Mauritsen T, Palmer MD, Watanabe M, Wild M, Zhang H (2021) The Earth’s Energy Budget, Climate Feedbacks, and Climate Sensitivity; Chapter 7; to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA.
Gao M, Carmichael GR, Wang Y, Saide PE, Yu M, Xin J, Liu Z, Wang Z (2016) Modeling study of the 2010 regional haze event in the North China Plain. Atmos Chem Phys 16(3):1673–1691
Gao M, Han Z, Tao Z, Li J, Kang JE, Huang K, Dong X, Zhuang B, Li S, Ge B, Wu Q, Lee HJ, Kim CH, S Fu J, Wang T, Chin M, Li M, Woo JH, Zhang Q, Chen Y, Wang Z, Carmichael GR (2020) Air quality and climate change, Topic 3 of the Model Inter-Comparison Study for Asia Phase III (MICS-Asia III) - Part 2: Aerosol radiative effects and aerosol feedbacks. Atmos Chem Phys 20(2):1147–1161
Grell GA, Freitas SR (2014) A scale and aerosol aware stochastic convective parameterization for weather and air quality modeling. Atmos Chem Phys 14:5233–5250
Guenther A, Karl T, Harley P, Weidinmyer C, Palmer PI, Geron C (2006) Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature). Atmos Chem Phys 6:3181–3210
Han Z, Ueda H, Matsuda K, Zhang R, Arao K, Kanai Y, Hasome H (2004) Model study on particle size segregation and deposition during Asian dust events in March 2002. 109:1–25.
Hashimoto A, Murakami M, Kato T, Muroi C, Yoshizaki M, Hayashi S (2004) Improvement of microphysical parameterization in a Japan Meteorological Agency Nonhydrostatic Model with a high resolution and its effect on simulation result. Research Activities in Atmospheric and Oceanic Modeling/WMO 34, 4-11–4-12. https://wgne.net/bluebook/uploads/2004/individual-articles/04_Hashimoto_Akihiro_WMO03_ahashimo.pdf. Accessed 10 Feb 2026
Hayashida S (2023) Tackling air pollution from agricultural residue burning: The Aakash project: Challenge for reduction of rice-stubble burning in the Indian Punjab region. Glob Environ Res 27(1):3–11
Hess M, Koepke P, Schult I (1998) Optical Properties of Aerosols and Clouds: The software package OPAC. Bull Am Meteorol Soc 79(5):831–44.
Iacono MJ, Delamere JS, Mlawer EJ, Shephard MW, Clough SA, Collins WD (2008) Radiative forcing by long-lived greenhouse gases: Calculations with the AER radiative transfer models. J Geophys Res Atmos 113:D13103
Ishida J, Aranami K, Kawano K, Matsubayashi K, Kitamura Y, Muroi C (2022) ASUCA : The JMA Operational Non-hydrostatic Model. J Meteor Soc Japan 100(5):3–6.
Jacobson MZ, Kaufman YJ, Rudich Y (2007) Examining feedbacks of aerosols to urban climate with a model that treats 3-D clouds with aerosol inclusions. J Geophys Res Atmos 112(24):D24205
Janjic ZI (1994) The step-mountain eta coordinate model: Further developments of the convection, viscous sublayer, and turbulence closure schemes. Mon Wea Rev 122:927–945
JMA (2008) Japan Meteorological Agency’s Non-Hydrostatic Model II, Suuchi Yohoka Hokoku Bessatsu (separate volume of annual report of Numerical Prediction Division), No. 54, 265 pp (in Japanese)
JMA (2013) Outline of the operational numerical weather prediction at the Japan Meteorological Agency. https://www.jma.go.jp/jma/jma-eng/jma-center/nwp/outline2013-nwp/index.htm. Accessed 10 Feb 2026.
Kain JS, Fritsch JM (1993) Convective parameterization for mesoscale models: the Kain-Fritsch scheme. The representation of cumulus convection in numerical models. Meteorol Monogr 24:165–170
Kaiser JW, Heil A, Andreae MO, Benedetti A, Chubarova N, Jones L, Morcrette J, Razinger M (2012) Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power. Biogeosciences, 9:527–554
Kajino M. (2011) MADMS: Modal Aerosol Dynamics model for multiple Modes and fractal Shapes in the free-molecular and near-continuum regimes. J Aerosol Sci 42:224–248
Kajino M, Ueda H, Han Z, Kudo R, Inomata Y, Kaku H (2017) Synergy between air pollution and urban meteorological changes through aerosol-radiation-diffusion feedback―A case study of Beijing in January 2013. Atmos Environ 171:98–110
Kajino M, Deushi M, Sekiyama TT, Oshima N, Yumimoto K, Tanaka TY, Ching J, Hashimoto A, Yamamoto T, Ikegami M, Kamada A, Miyashita M, Inomata Y, Shima S-I, Takami A, Shimizu A, Hatakeyama S. (2019) NHM-Chem, the Japan meteorological agency’s regional meteorology – chemistry model: Model evaluations toward the consistent predictions of the chemical, physical, and optical properties of aerosols. J Meteorol Soc Japan 97(2):337–374
Kajino M, Deushi M, Sekiyama TT, Oshima N, Yumimoto K, Tanaka TY, Ching J, Hashimoto A, Yamamoto T, Ikegami M, Kamada A, Miyashita M, Inomata Y, Shima SI, Khatri P, Shimizu A, Irie H, Adachi K, Zaizen Y, Igarashi Y, Ueda H, Maki T, Mikami, M (2021) Comparison of three aerosol representations of NHM-Chem (v1.0) for the simulations of air quality and climate-relevant variables. Geosci Model Dev 14(4):2235–2264
Kajino M, Kamada A, Tanji N, Kuramochi M (2022) Quantitative influences of interannual variations in meteorological factors on surface ozone concentration in the hot summer of 2018 in Japan. Atmos Environ X 16:100191
Kajino M, Ishijima K, Ching J, Yamaji K, Ishikawa R, Kajikawa T, Singh T, Nakayama T, Matsumi Y, Kojima K, MacHida T, Maki T, Patra PK, Hayashida S (2025) Impact of post-monsoon crop residue burning on PM2.5 over northern India: optimizing emissions using a high-density in situ surface observation network. Atmos Chem Phys 25(13):7137–7160
Kajino M, Orikasa N, Kudo R, Shimizu A, Osada K, Kayaba S, Kajikawa T, Ishikawa R, Yumimoto K (2026) A practical method for evaluating 3D aerosol physics and chemistry models with size-resolved aerosol measurement data: Application to NHM-Chem v2.0. to be submitted Geosci Model Dev
Kanji ZA, Ladino LA, Wex H, Boose Y, Burkert-Kohn M, Cziczo DJ, Krämer M. (2017) Overview of ice nucleating particles. Meteorol Monogr 58:1.1–1.33
Keita SA, Girard E, Raut JC, Leriche M, Blanchet JP, Pelon J, Onishi T, Cirisan A (2020) A new parameterization of ice heterogeneous nucleation coupled to aerosol chemistry in WRF-Chem model version 3.5.1: Evaluation through ISDAC measurements. Geosci Model Dev 13(11):5737–5755
Kerminen VM, Kulmala M (2002) Analytical formulae connecting the “real” and the “apparent” nucleation rate and the nuclei number concentration for atmospheric nucleation events. J Aerosol Sci 33(4):609–622
Kulmala M, Kokkonen T, Ezhova E, Baklanov A, Mahura A, Mammarella I, Bäck J, Lappalainen HK, Tyuryakov S, Kerminen VM, Zilitinkevich S, Petäjä T (2023) Aerosols, clusters, greenhouse gases, trace gases and boundary-layer dynamics: On feedbacks and interactions. Boundary-Layer Meteorol 186(3):475–503
Kobayashi S, Ota Y, Harada Y, Ebita A, Moriya M, Onoda H, Onogi K, Kamahori H, Kobayashi C, Endo H, Miyaoka K, Kiyotoshi T (2015) The JRA-55 reanalysis: General specifications and basic characteristics. J Meteorol Soc Japan 93(1):5–48
Kurokawa J, Ohara T. (2020) Long-term historical trends in air pollutant emissions in Asia: Regional Emission inventory in ASia (REAS) version 3. Atmos Chem Phys 20:12761–12793
Li J, Dong H, Zeng L, Zhang Y, Shao M, Wang Z, Sun Y, Fu P (2015) Exploring possible missing sinks of nitrate and its precursors in current air quality models―A case simulation in Pearl River delta of China using an observation-based box model. Sci Online Lett Atmos 11:124–128
Li M, Wang T, Xie M, Zhuang B, Li S, Han Y, Chen P (2017) Impacts of aerosol-radiation feedback on local air quality during a severe haze episode in Nanjing megacity, eastern China. Tellus, 69(1):1339548
Li J, Han Z, Wu Y, Xiong Z, Xia X, Li J, Liang L, Zhang R. Aerosol radiative effects and feedbacks on boundary layer meteorology and PM2.5 chemical components during winter haze events over the Beijing-Tianjin-Hebei region. Atmos. Chem. Phys. 2020;20(14):8659–90.
Liu T, Mickley LJ, Singh S, Jain M, Defries RS, Marlier ME (2020) Crop residue burning practices across north India inferred from household survey data : Bridging gaps in satellite observations. Atmos Environ X 8:100091
Lohmann U, Diehl K (2006) Sensitivity studies of the importance of dust ice nuclei for the indirect aerosol effect on stratiform mixed-phase clouds. J Atmos Sci 63(3):968–982
Mangaraj P, Matsumi Y, Nakayama T, Biswal A, Yamaji K, Araki H, Yasutomi N, Takigawa M, Patra PK, Hayashida S, Sharma A, Dimri AP, Dhaka SK, Bhatti MS, Kajino M, Mor S, Khaiwal R, Bhardwaj S, Vazhathara VJ, Kunchala RK, Mandal TK, Misra P, Singh T, Vatta K, Mor S (2025) Weak coupling of observed surface PM2.5 in Delhi-NCR with rice crop residue burning in Punjab and Haryana. npj Clim Atmos Sci 8(1):18
Meyers MP, Demott PJ, Cotton WR (1992) New primary ice-nucleation parameterizations in an explicit cloud model. J Appl Meteorol 31:708–721
Morrison H, Thompson G, Takarskii V (2009) Impact of cloud microphysics on the development of trailing stratiform precipitation in a simulated squall line: Comparison of one- and two-moment schemes. Mon Wea Rev 137:991–1007
Nakata M, Kajino M, Sato Y (2021) Effects of mountains on aerosols determined by AERONET/DRAGON/J-ALPS measurements and regional model simulations. Earth Space Sci 8:1–15.
Nakayama T, Matsumi Y, Kawahito K, Watabe Y (2018) Development and evaluation of a palm-sized optical PM2.5 sensor. Aerosol Sci Tech 52: 2–12
Nishizawa S, Yashiro H, Sato Y, Miyamoto Y, Tomita H (2015) Influence of grid aspect ratio on planetary boundary layer turbulence in large-eddy simulations. Geosci Model Dev 8:3393–3419
Petters MD, Kreidenweis SM (2007) A single parameter representation of hygroscopic growth and cloud condensation nucleus activity. Atmos Chem Phys 7:1961–1971
Pleim JE, Chang JS. (1992) A non-local closure model for vertical mixing in the convective boundary layer. Atmos Environ 26A(6):965–981
Qian Y, Gong D, Fan J, Ruby Leung L, Bennartz R, Chen D, Wang W (2009) Heavy pollution suppresses light rain in China: Observations and modeling. J Geophys Res Atmos 114(15):D00K02
Rathore J, Ganguly D, Singh V, Gupta M, Vazhathara VJ, Biswal A, Kunchala RK, Patra PK, Sahu LK, Gani S, Dey S (2025) Characteristics of haze pollution events during biomass burning period at an upwind site of Delhi. J Geophys Res Atmos 130:e2024JD042347
Saito K, Fujita T, Yamada Y, Ishida Y, Kumagai Y, Aranami K, Ohmori S, Nagasawa R, Kumagai S, Muroi C, Kato T, Eito H, Yamazaki Y (2006) The Operational JMA Nonhydrostatic Mesoscale Model. Mon Wea Rev 134:1266–1298
Saito K, Ishida J, Aranami K, Hara T, Segawa T, Narita M, Honda Y (2007) Nonhydrostatic atmospheric models and operational development at JMA. J. Meteor Soc Japan 85B:271–304
Sakai T, Nagai T, Zaizen Y, Mano Y (2010) Backscattering linear depolarization ratio measurements of mineral, sea-salt, and ammonium sulfate particles simulated in a laboratory chamber. Appl Opt 49(23):4441–4449
Sato Y, Kajino M, Hayashi S, Wada R (2023) A numerical study of lightning-induced NOx and formation of NOy observed at the summit of Mt. Fuji using an explicit bulk lightning and photochemistry model. Atmos Environ X 18:100218
Sato Y, Kajino M, Hayashi S, Wada R (2024) Corrigendum to “A numerical study of lightning-induced NOx and formation of NOy observed at the summit of Mt. Fuji using an explicit bulk lightning and photochemistry model” [Atmos. Environ. X 18. (2023) 100218] Atmos Environ X 22:100231
Sato Y, Nishizawa S, Yashiro H, Miyamoto Y, Kajikawa Y, Tomita H. (2015) Impacts of cloud microphysics on trade wind cumulus: which cloud microphysics processes contribute to the diversity in a large eddy simulation? Prog Earth Planet Sci 2:23
Sekiyama TT, Kajino M (2022) Simultaneous data assimilation of meteorological fields and atmospheric concentration fields using variable localization in the ensemble Kalman filter. Proc Inst Stat Math 70(2):165–179 (in Japanese)
Singh T, Matsumi Y, Nakayama T, Hayashida S, Patra PK, Yasutomi N, Kajino M, Yamaji K, Khatri P, Takigawa M, Araki H, Kurogi Y, Kuji M, Muramatsu K, Imasu R, Ananda A, Arbain AA, Ravindra K (2023) Very high particulate pollution over northwest India captured by a high density in situ sensor network. Sci Rep 13:13201
Skamarock WC, Klemp JB, Gill DO, Powers JG, Duda MG, Barker DM (2019) A Description of the Advanced Research WRF Model Version 4, NCAR Technical Notes NCAR / TN-55 6 + STR
Suzuki T, Iwata A, Yamashita K, Kuo WC, Kobayashi H, Orikasa N, Misumi R, Kusaka H, Shima S, Kajino, M (2026) Seasonal variation of atmospheric aerosol particles and ice-nucleating particles at Mt. Tsukuba. SOLA in review
Szopa S, Naik V, Adhikary B, Artaxo P, Berntsen T, Collins WD, Fuzzi S, Gallardo L, Kiendler-Scharr A, Klimont Z, Liao H, Unger N, Zanis P (2021) Short-lived Climate Forcers; Chapter 6; to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA.
Takigawa M, Patra PK, Matsumi Y, Dhaka SK, Nakayama T, Yamaji K, Kajino M, Hayashida S (2020) Can Delhi’ s pollution be affected by crop fires in the Punjab region? 16:86–91
Tanaka TY, Ogi A (2017) Update of Japan Meteorological Agency’s global mineral dust operational forecast model. Sokko-Jihou 84:109-128 (in Japanese)
Thompson G, Eidhammer T (2014) A study of aerosol impacts on clouds and precipitation development in a large winter cyclone. J Atmos Sci 71(10):3636–3658
Uno I, Ueda H, Wakamatsu S (1989) Numerical modeling of the nocturnal urban boundary layer. Boundary-Layer Meteorol 49:77–98.
Vaezi RB, Martin MR, Hosseinpour F (2025) Impacts of wildfire smoke aerosols on radiation, clouds, precipitation, climate, and air quality. Atmos Environ X 26:100322
Yamagami A, Kajino M, Maki T (2022) Statistical evaluation of the temperature forecast error in the lower-level troposphere on short-range timescales induced by aerosol variability. J Geophys Res Atmos 127(13):e2022JD036595
Yoshida M, Murakami H (2021) Algorithm theoretical basis document of aerosol properties for GCOM-C/SGLI. https://suzaku.eorc.jaxa.jp/GCOM_C/data/ATBD/ver3/V3ATBD_A3AB_ARNP_MYoshida_20220106.pdf. Accessed 26 Jan 2026.
Yumimoto K, Takemura T (2013) The SPRINTARS version 3.80/4D-Var data assimilation system: Development and inversion experiments based on the observing system simulation experiment framework. Geosci Model Dev 6(6):2005–2022.
Zhang Y (2008) Online-coupled meteorology and chemistry models: History, current status, and outlook. Atmos Chem Phys 8(11):2895–2932.
Zhang Y, Wen XY, Jang CJ. Simulating chemistry-aerosol-cloud-radiation-climate feedbacks over the continental U.S. using the online-coupled Weather Research Forecasting Model with chemistry (WRF/Chem). Atmos. Environ. [Internet]. Elsevier Ltd; 2010;44(29):3568–82. Available from: http://dx.doi.org/10.1016/j.atmosenv.2010.05.056
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Kajino, Mizuo
Makoto Deushi
Akihiro Hashimoto
Rei Kudo
Ryoji Nagasawa
Tsuyoshi Thomas Sekiyama
Tomoki Kajikawa
Satoko Kayaba
Yukari Hara
Keiya Yumimoto
Dilip Ganguly
Sachiko Hayashida
Takashi Maki
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